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Thermally Induced Local Failures in Quasi-One-Dimensional Systems: Collapse in Carbon Nanotubes, Necking in Nanowires and Opening of Bubbles in DNA

机译:准一维系统中的热致局部失效:   碳纳米管塌陷,纳米线缩颈和气泡开口   脱氧核糖核酸

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摘要

We present a general framework to explore thermally activated failures inquasi one dimensional systems. We apply it to the collapse of carbon nanotubes,the formation of bottlenecks in nanowires, both of which limit conductance, andthe opening of local regions or "bubbles" of base pairs in strands of DNA thatare relevant for transcription and danaturation. We predict an exponentialbehavior for the probability of the opening of bubbles in DNA, the averagedistance between flattened regions of a nanotube or necking in a nanowire as amonotonically decreasing function of temperature, and compute a temperaturebelow which these events become extremely rare. These findings are difficult toobtain numerically, however, they could be accessible experimentally.
机译:我们提出了一个一般的框架来探讨准一维系统的热激活故障。我们将其应用于碳纳米管的崩溃,纳米线中瓶颈的形成(这两者都限制了电导)以及与转录和变性相关的DNA链中碱基对的局部区域或“气泡”的开放。我们预测DNA中气泡打开的概率,纳米管的扁平区域之间或纳米线颈缩之间的平均距离作为温度的单调递减函数的指数行为,并计算低于这些事件变得极为罕见的温度。这些发现很难从数字上获得,但是,它们可以通过实验获得。

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